Abstract
The US Department of Energy (DOE) manages an inventory of materials that contains a range of long-lived radioactive isotopes that were produced from the 1960s through the 1980s by irradiating targets in production reactors to produce special heavy isotopes for DOE programmatic use, scientific research, and industrial and medical applications. Oak Ridge National Laboratory (ORNL) used many of these materials as feedstock in the calutron Electromagnetic Isotope Enrichment Facility (EIEF), one of only two facilities in the world with capabilities to enrich radioisotopes in multigram quantities. Both the production reactors and enrichment facilities have been shut down, and many of these unique materials will never be produced again. ORNL maintains a major portion of the United States’ inventory of these materials and uses them in DOE’s center for production, storage, and distribution of transuranium isotopes (plutonium through californium) to the user community. The US inventory of enriched actinides is being depleted, and attempts for over a decade to obtain critical supplies from foreign sources have been unsuccessful. Significant strides have been made recently in the development of new and improved enrichment technologies to replace the previous electromagnetic separations techniques. This paper summarizes the US’s need for production of high-purity enriched actinides by national security, nuclear nonproliferation, and basic research programs.
