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Neutron Scattering Studies of Spin-Phonon Hybridization and Superconducting Spin-Gaps in the High Temperature Superconductor ...

Publication Type
Journal
Journal Name
Physical Review B
Publication Date
Page Number
094416
Volume
93

We present time-of-
ight neutron-scattering measurements on single crystals of La2-xBaxCuO4 (LBCO) with 0 < x < 0.095 and La2-xSrxCuO4 (LSCO) with x = 0.08 and 0.11. This range of dopings spans much of the phase diagram relevant to high temperature cuprate superconductivity, ranging from insulating, three dimensional commensurate long range antiferromagnetic order for x <= 0.02 to two dimensional (2D) incommensurate antiferromagnetism co-existing with superconductivity for x >= 0.05. Previous work on lightly doped LBCO with x = 0.035 showed a clear resonant enhancement of the inelastic scattering coincident with the low energy crossings of the highly dispersive spin excitations and quasi-2D optic phonons. The present work extends these measurements across the phase diagram and shows this enhancement to be a common feature to this family of layered quantum magnets. Furthermore we show that the low temperature, low energy magnetic spectral weight is substantially larger for samples with non-superconducting ground states
relative to any of the samples with superconducting ground states. Spin gaps, suppression of low energy magnetic spectral weight, are observed in both superconducting LBCO and LSCO samples, consistent with previous observations for superconducting LSCO