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Chemically Driven Nanoscopic Magnetic Phase Separation at the SrTiO(3)(001)/La(1-x)Sr(x)CoO(3) Interface...

Publication Type
Journal
Journal Name
Advanced Materials
Publication Date
Page Numbers
2711 to 2715
Volume
23
Issue
24

The degradation in magnetic properties in very thin film complex oxides is studied using SrTiO(3)(001)/La(1-x)Sr(x)CoO(3), providing unequivocal evidence for nanoscopic interfacial magnetic phase separation. Electron microscopy and spectroscopy reveal that this occurs due to inhomogeneity in local hole doping, driven by subtle, depthwise variations in the Sr and O stoichiometry. Simple thermodynamic and structural arguments for the origin of these variations are provided.