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Inelastic neutron scattering study of a nonmagnetic collapsed tetragonal phase of CaFe2As2: Evidence of the impact of spin f...

Publication Type
Journal
Journal Name
Physical Review Letters
Publication Date
Page Number
227002
Volume
111
Issue
22

The relationship between antiferromagnetic spin fluctuations and superconductivity has become a central
topic of research in studies of superconductivity in the iron pnictides. We present unambiguous evidence of the
absence of magnetic fluctuations in the non-superconducting collapsed tetragonal phase of CaFe2As2 via inelas-
tic neutron scattering time-of-flight data, which is consistent with the view that spin fluctuations are a necessary
ingredient for unconventional superconductivity in the iron pnictides. We demonstrate that the collapsed tetrag-
onal phase of CaFe2As2 is non-magnetic, and discuss this result in light of recent reports of high-temperature
superconductivity in the collapsed tetragonal phase of closely related compounds.