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Unusual Phonon Heat Transport in α−RuCl3: Strong Spin-Phonon Scattering and Field-Induced Spin Gap...

Publication Type
Journal
Journal Name
Physical Review Letters
Publication Date
Page Number
117204
Volume
120
Issue
11

The honeycomb Kitaev-Heisenberg model is a source of a quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. Here we unveil the highly unusual low-temperature heat conductivity κ of α−RuCl3, a prime candidate for realizing such physics: beyond a magnetic field of Bc≈7.5  T, κ increases by about one order of magnitude, both for in-plane as well as out-of-plane transport. This clarifies the unusual magnetic field dependence unambiguously to be the result of severe scattering of phonons off putative Kitaev-Heisenberg excitations in combination with a drastic field-induced change of the magnetic excitation spectrum. In particular, an unexpected, large energy gap arises, which increases linearly with the magnetic field, reaching remarkable ℏω0/kB≈50  K at 18 T.